Bench X-ray microtomography of water-salt solution/oil injected into samples of the Botucatu formation
DOI:
https://doi.org/10.5433/1679-0375.2022v43n2p199Keywords:
X-ray microtomography, Fluids, Microstructure, sandstoneAbstract
This paper provides a report on the utilization of the X-ray microtomography to obtain images of the internal microstructure of natural sandstone samples from the Botucatu Formation. Its primary objective was to identify the different phases of fluids when injected into the samples to evaluate the various phases through grayscale histograms obtained from 2-D images, quantification of fluid phases, and generation of 3-D images of them. The fluids used in the experiments comprised one type of commercial oil, one type of industrial oil, and an water-salt solution. Quantitative results from 2-D and 3-D analyzes are presented and compared to the volume of injected solution and the measured volume. The phase size distributions indicated which pore radii had a more relevant participation in the percolation of fluids through the samples. Projections in conjunction with 2-D images and profiles of average percentages of air-filled pores indicated the occurrence of preferential percolation flow paths. The 2-D images allowed the measurement of the contact angle between the phases present in the sample containing industrial oil. Different measurements taken from the sample containing commercial oil showed capillary effects indicated by the average percentage profiles of air-filled pores in the 2-D images.
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References
Bear, J. (1988). Dynamics of fluids in porous media, x ed. Dover Publications, Dover, 802 p.
Brown, K., Schlüter, S., Sheppard, A., Wildeschild, D. (2014). On the challenges of measuring interfacial characteristics of three-phase fluid flow with x-ray microtomography. Journal of Microscopy, 253: 171-182, https://doi.org/10.1111/jmi.12106 DOI: https://doi.org/10.1111/jmi.12106
Bultreys, T., Boever, W. D., Cnudde, V. (2016). Imaging and image-based fluid transport modeling at the pore scale in geological materials: A practical introduction to the current state-of-the-art. Earth-Science Reviews, 155: 93-128, http://dx.doi.org/10.1016/j.earscirev.2016.02.001 DOI: https://doi.org/10.1016/j.earscirev.2016.02.001
Cardoso, O. R., Balaban, R. C. (2015). Comparative study between Botucatu and Berea sandstone properties. Journal of South American Earth Sciences, 62: 58-69, http://dx.doi.org/10.1016/j.jsames.2015.04.004 DOI: https://doi.org/10.1016/j.jsames.2015.04.004
Costa, A. A., Trivedi, J., Soares, J., Rocha, P., Costa, G.,Embiruçu, M. (2020). An experimental evaluation of low salinity water mechanisms in a typical Brazilian sandstone and light crude oil with low acid/basic number. Fuel, 273: 1-18, https://doi.org/10.1016/j.fuel.2020.117694 DOI: https://doi.org/10.1016/j.fuel.2020.117694
Fagundes, J. R. T., Zuquette, L. V. (2011). Sorption behavior of the sandy residual unconsolidated material from the sandstones of the Botucatu Formation, the mais aquifer of Brazil. Environmental Earth Science, 62: 831-845, http://doi.org/10.1007/s12665-010-0570-y DOI: https://doi.org/10.1007/s12665-010-0570-y
Fernandes, J. S., Appoloni, C. R., Fernandes, C. P. (2019). Siltstone and sandstone pore space by X-ray microtomography. Soils and Rocks, 42(3): 281-288, https://doi.org/ 10.28927/SR.423281 DOI: https://doi.org/10.28927/SR.423281
Fogden, A., Middleton, J., McKay, T., Latham, S., Marathe, R., Turner, M., Sheppard, A., Howard, J. J., Lane, F. D. (2014). 3D mapping of pore and organic matter distributions in unconventional reservoir utilizing a digital rocks approach. Proc. International Symposium, Society of Core Analysts, Avignon, v. A042, pp. 1-12.
Goldstein, L., Prasher, S. O., Ghoshal, S. (2007). Three-dimensional visualization and quantification of non-aqueous phase liquid volumes in natural porous media using a medical X-ray Computed Tomography scanner. Journal of Contaminant Hydrology, 93: 96-110, http://dx.doi.org/10.1016/j.jconhyd.2007.01.013, 2007 DOI: https://doi.org/10.1016/j.jconhyd.2007.01.013
Ketcham, R. A., Carlson, W. D. (2001). Acquisition, optimization and interpretation of X-ray computed tomographic imagery: applications to the geosciences. Computers & Geosciences, 27: 381-400, http://dx.doi.org/10.1016/S0098-3004(00)00116-3 DOI: https://doi.org/10.1016/S0098-3004(00)00116-3
Kumar, M., Senden, T., Knackstedt, M., Latham, S., Pinczewski, V., Sok, R. M., Sheppard, A. P., Turner, M. L. (2009). Imaging of pore scale distribution of fluids and Wettability, Petrophysics Journal, 4: 311-321, http://hdl.handle.net/1885/52974
Marques, L. C., Appoloni, C. R., Fernandes, C. P. (2011). Porosity Study of Synthetic Sandstones by Non-Destructive Nuclear Techniques. Materials Research, 14 (3): 1-9, http://dx.doi.org/10.1590/S1516-14392011005000048 DOI: https://doi.org/10.1590/S1516-14392011005000048
Marques, L. C., Appoloni, C. R. (2015). Quantification of fluids in a glass-bead matrix using X-ray microtomography. Micron, 75: 35-43, http://dx.doi.org/10.1016/j.micron.2015.03.001 DOI: https://doi.org/10.1016/j.micron.2015.03.001
Moreira, A. C., Appoloni, C. R., Mantovani, I. F., Fernandes, J. S., Marques, L. C., Nagata, R., Fernandes, C. P. (2012). Effects of manual threshold setting on image analysis results of a sandstone sample structural characterization by X-ray microtomography. Applied Radiationand Isotopes, 70: 937-941, http://dx.doi.org/10.1016/j.apradiso.2012.03.001 DOI: https://doi.org/10.1016/j.apradiso.2012.03.001
Oliveira, E. P., Santelli, R. E., Cassella, R. J. (2008). Combined use of Pd and HF as chemical modifiers for the determination of total chromium in produced waters from petroleum exploration by ET AAS. Microchemical Jounal, 89: 116-122, http://dx.doi.org/10.1016/j.microc.2008.01.002 DOI: https://doi.org/10.1016/j.microc.2008.01.002
Pak, T., Butler, I. B., Geiger, S., Vandijke, M. I. J., Sorbie, K. S. (2015). Doplet fragmentation: 3D imaging of a previously unidentified pore-scale process during multiphase flow in porous media. PNAS, 112 (7): 1947-1952, www.pnas.org/lookup/suppl/doi:10.1073/pnas.1420202112/-/DCSupplemental. DOI: https://doi.org/10.1073/pnas.1420202112
PETROBRAS. Tecnologia e Pesquisa available at http://www.petrobras.com.br/pt/energia-e-tecnologia/tecnologia-e-pesquisa and download on Octuber 8th 2019.
Rao, S. M., Sivachidambaram, S. (2013). Characterization and iodide adsorption behavior of HDPY + modified bentonite. Environmental Earth Sciences, 68: 559-566, http://dx.doi.org/10.1007/s12665-012-1759-z DOI: https://doi.org/10.1007/s12665-012-1759-z
Rattanasak, U., Kendall, K. (2005). Pore structure of cement/pozzolan composites by X-ray microtomography. Cement and Concrete Research, 35: 637-640, http://dx.doi.org/10.1016/j.cemconres.2004.04.022 DOI: https://doi.org/10.1016/j.cemconres.2004.04.022
Riebe, B., Dultz, S., Bunnenberg, C. (2005). Temperature effects on iodine adsorption on organo-clay minerals I. Influence of pretreatment and adsorption temperature. Applied Clay Science, 28: 9-16, http://dx.doi.org/10.1016/j.clay.2004.01.004 DOI: https://doi.org/10.1016/j.clay.2004.01.004
Saetre, C., Tjugum, S. (2014). Tomographic segmentation in multiphase flow measurement. Radiation Physics and Chemestry, 95: 420-423, http://dx.doi.org/10.1016/j.radphyschem.2013.03.025 DOI: https://doi.org/10.1016/j.radphyschem.2013.03.025
Sezgin, M., Sankur, B. (2004). Survey over image thresholding techniques and quantitative performance evaluation. Journal of Electronic Imaging, 13(1): 146-165, http://dx.doi.org/10.1117/1.1631316 DOI: https://doi.org/10.1117/1.1631315
Vinegar, H. J., Wellington, S. L. (1987). Tomographic Imaging of Three-Phase Flow Experiments. Rev. Sci. Instrum, 58(1): 96-107, http://dx.doi.org/10.1063/1.1139522 DOI: https://doi.org/10.1063/1.1139522
Wildenschild, D., Culligan, K. A., Christensen, B. S. B. (2004). Application of x-ray microtomography to environmental fluid flow. Proc. 49th Annual Meeting, Optical Science and Technology. Denver, v. 5535, (Develpoments in X-Ray IV), http://dx.doi.org/10.1117/12.559056 DOI: https://doi.org/10.1117/12.559056
Wildenschild, D., Hopmans, J. W., Kent, A. J. R. (2005). Quantitative Analysis of Flow Process in a Sand Using Synchrotron-Based X-ray Microtomography. Vadose Zone Journal, 4: 112-126, http://dx.doi.org/10.2113/4.1.112 DOI: https://doi.org/10.2113/4.1.112
Zeng, Q., Li, K., Fen-Chong, T., Dangla, P. (2012). Analysis of pore structure, contact angle and pore entrapment of blended cement pastes from mercury porosimetry data. Cement and Concrete Composites, 34(9): 1053-1060, http://dx.doi.org/10.1016/j.cemconcomp.2012.06.005 DOI: https://doi.org/10.1016/j.cemconcomp.2012.06.005
Zuquette, L. V., Palma, J. B., Pejon, O. J. (2006). Initial assessment of the infiltration and overland flow for different rainfall events in land constituted of sandstones of the Botucatu Formation (Guarani Aquifer), State of São Paulo, Brazil. Environ. Geol., 50: 371-387, http://dx.doi.org/10.1007/s00254-006-0216-2 DOI: https://doi.org/10.1007/s00254-006-0216-2
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